Artemis

Artemis is the CLF’s facility for ultrafast science, using extreme ultraviolet (XUV) pulses produced through high-harmonic generation for time-resolved photoelectron spectroscopy, photoemission, transient absorption and ptychographic imaging.

Facility Overview

1 kHz Ti:sapphire laser system

  • ​twin 8 mJ, 30fs pulses at 1kHz
  • few-cycle laser pulses at 1800nm
  • tuneable pulses from 235nm to 15 microns

100 kHz IR system​, with outputs at 1700nm and 3000nm.​​​

Experiments on Artemis use high harmonic generation (HHG) to investigate ultrafast dynamics in experiments on gas, liquidand solid materials. The spatial coherence of the XUV radiation is also leveraged to perform coherent diffractive imaging techniques. Artemis is based on high-repetition rate, widely tuneable femtosecond laser sources, and ultrafast XUV (10 to 150eV) pulses produced through HHG. The facility comprises two ultrafast laser systems and three in-vacuum XUV beamlines, with specialised end-stations to support user experiments.

Applications

Environment: atmospheric chemistry
Advanced materials: photovoltaics and photocatalysts 
Quantum technologies: 2D materials 
Semiconducting transition metal dichalcogenides (TMDCs)

In the atmosphere, sunlight triggers photochemical reactions that can break down chemicals to form new products or free radicals. Recent experiments on Artemis have studied several molecules which are atmospheric pollutants, using ultraviolet pulses to initiate the photochemical reaction and then XUV to study its evolution in time and final photoproducts.

Light harvesting devices need to combine strong absorption in the visible spectral range with efficient ultrafast charge separation. Artemis can directly measure change in electron populations, to obtain information on the charge separation and recombination times. 

The recombination pathways of charge carriers are also important to photocatalysis because they determine the lifetime of chemically active sites and hence the catalytic efficiency.

New emergent phenomena often arise from the competition or cooperation of electronic phases in quantum materials. Understanding them can guide the design of novel material functionalities, such as unusual electronic properties. 

2D materials have the potential to result in devices that are smaller, run faster, and consume less power, as well as offering a wealth of other potentials such as foldable, flexible, transparent electronics. 

 In 2013, the first direct measurements of ultrafast electronic dynamics in graphene – recognised as the world’s first 2D material – were made using Artemis.

The resulting papers now have over 1,000 citations between them.

The high degree of control over the electronic properties and strong light-matter interactions in semiconducting TMDCs make them promising candidates for novel applications in photonics, optoelectronics and spintronics. For example, we can use laser pulses to switch the material from an insulating state to a metal state, on a sub-ps timescale, and directly measure the change in electronic band structure while this happens.

Technical specifications

Artemis has two high-repetition rate and high average power femtosecond laser systems, three vacuum beamlines for XUV generation and filtering, and four end-stations for user experiments.

Laser system 1: Fastlite OPCPA 

System 1 is a 100kHz infrared laser system from Fastlite, producing >20W (200µJ) in 50fs pulses at 1700nm, and >5W in 60fs pulses at 3000nm. The system is based on Optical Parametric Chirped Pusle Amplification (OPCPA), pumped by a 225-W Yb:YAG thin-disk regenerative amplifier from Trumpf Scientific, based on an industrial micro-machining system. The OPCPA has two modes of output. One offers <50fs pulses at 1700nm and <60fs pulses 3000nm, and the other offers broader tuning ranges (1,430 to 1,850nm and 2,330 to 3,680nm) but slightly longer pulses (80 to 180fs).  

The system also has a multi-pass Herriott cell to generate short pulses at 1030nm to be used for high-harmonic generation (HHG). Alternatively, the infrared can be split and a portion used for HHG whilst the rest is used for the optical pump. 

Laser system 2: Light Conversion system 

System 2 is a 100kHz laser system from Light Conversion. It consists of three optically synchronised Yb:KGW lasers (Light Conversion Carbides) using a common oscillator. One 200W Carbide laser is used to drive a hollow core fibre (FewCycle) to generate >150W of <50fs, 1030nm light which is used for high-harmonicgeneration. A second 200W Carbide is used to drive one of two Orpheus optical parametric amplifiers to produce short pulses which are continuously tuneable from 235nm to 10 microns. A third 80W Carbide laser will be post-compressed or used for frequency mixing. 

High harmonic light sources 

Artemis produces coherent, femtosecond pulses of XUV through HHG in a gas target. A laser is focused to an intensity of approximately 1014 Wcm-2 in a differentially pumped gas cell and up to one part in 106 of the energy is converted to short pulses of XUV radiation in the 8 to 120nm (10 to 150eV) range. The XUV pulses have a similar pulse-duration to the drive laser pulses (approximately 50fs) and are synchronised to them with sub-fs resolution.

Meet the team

Yu Zhang

Senior experimental scientist

Yu is a specialist in ultrafast laser photoelectron spectroscopy and low-dimensional quantum materials.

Tiffany Walmsley

Experimental Scientist

Experimental Scientist: Artemis, Central Laser Facility, 2024 to present

Sneha Banerjee

Senior Experimental Scientist

Senior Experimental Scientist: Artemis, Central Laser Facility, 2025 to present

Oliver Smith

Graduate laser scientist

Oliver joined Artemis in September 2024, where he works on the DynAMO extreme ultraviolet beamline and end station to facilitate gas phase ultra-fast spectroscopy experiments.​

James Thompson

Senior Experimental Scientist

Senior Experimental Scientist, AMO science programme: Artemis Facility, CLF, UK, 2023 to present

Emma Springate

Artemis Group Leader

Emma has led the Artemis group since it opened to users.

Bruce Weaver

Experimental Scientist

Experimental Scientist: Artemis, Central Laser Facility, 2024 to present.